(EBook PDF) Optical Multidimensional Coherent Spectroscopy 1st edition by Hebin Li, Bachana Lomsadze, Galan Moody, Christopher Smallwood, Steven Cundiff 0192657623 9780192657626 full chapters

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Product details:

ISBN-10 :  0192657623 

ISBN-13 :  9780192657626

Author: Hebin Li, Bachana Lomsadze, Galan Moody, Christopher Smallwood, Steven Cundiff 

This book provides an introduction to optical multidimensional coherent spectroscopy, a relatively new method of studying materials based on using ultrashort light pulses to perform spectroscopy. The technique has been developed and perfected over the last 25 years, resulting in multiple experimental approaches and applications to a broad array of systems ranging from atoms and molecules to solids and biological systems. Indeed, while this method is most often used by physical chemists, it is also relevant to materials of interest to physicists, which is the primary focus of this book. As well as an introduction to the method, the book also provides tutorials on the interpretation of the rather complex spectra that is broadly applicable across all subfields, and finishes with a survey of several emerging material systems and a discussion of future directions.

 

Optical Multidimensional Coherent Spectroscopy 1st Table of contents:

1. Basics of ultrafast spectroscopy
2. Basics of spectroscopy: linear versus nonlinear
3. Ultrashort pulses
4. Ultrafast nonlinear/coherent spectroscopy
5. The density matrix
6. Bloch sphere representation of quantum states
7. Introduction to multidimensional coherent spectroscopy
8. Concepts of multidimensional coherent spectroscopy
9. Coherent spectroscopy
10. Multidimensional coherent spectroscopy
11. Spectrum classification
12. Density matrix formalism and double-sided Feynman diagrams
13. Interpreting MDCS in the perturbative limit
14. Double-sided Feynman diagrams
15. Measured observables
16. Putting it all together
17. Case study: Two-level system
18. Phase matching
19. Two-dimensional infrared (2D IR) spectroscopy
20. Interpretation of multidimensional coherent spectra
21. Isolated two-level system
22. Inhomogeneously broadened ensemble of two-level systems
23. Gaussian inhomogeneity, constant homogeneous linewidth
24. Large inhomogeneity
25. Coherent coupling signatures
26. Incoherent coupling signatures
27. Doubly excited states and many-body interactions
28. Double-quantum spectra
29. Zero-quantum spectra
30. Three-dimensional coherent spectroscopy
31. Nonrephasing pathways and purely absorptive spectra
32. Finite-pulse effects
33. Mathematical formulations
34. Example spectra
35. Further applications
36. Experimental implementations
37. Experimental requirements and considerations
38. Precision and stability of time delays
39. Isolation of the signal
40. Detection of the signal
41. Overview of experimental approaches
42. Actively stabilized box geometry
43. Phase modulated collinear geometry
44. Comparison of different approaches
45. Data analysis
46. Multidimensional coherent spectroscopy of atomic ensembles
47. Single- and zero-quantum 2D spectra of atomic vapors
48. MDCS in optically thick samples
49. Probing many-body interactions with double-quantum 2D spectroscopy
50. Probing many-body correlations with multi-quantum 2D spectroscopy
51. Frequency comb-based multidimensional coherent spectroscopy
52. Introduction to frequency combs and dual-comb spectroscopy
53. Frequency comb-based four-wave-mixing spectroscopy
54. Frequency comb-based single-quantum 2D spectroscopy
55. Frequency comb-based double-quantum 2D spectroscopy
56. Tri-comb spectroscopy
57. Two-dimensional spectroscopy of semiconductor quantum wells
58. Introduction to semiconductor optics
59. Many-body signatures in one-quantum 2D spectra
60. Many-body signatures in double- and multi-quantum 2D spectra
61. Two-dimensional spectroscopy of coupled quantum wells
62. Quantum well exciton-polaritons in microcavities
63. Three-dimensional coherent spectroscopy
64. Fifth-order 3D infrared spectroscopy
65. Fifth-order 3D electronic spectroscopy
66. Third-order 3D electronic spectroscopy
67. Three-dimensional spectra of atomic vapors
68. Three-dimensional spectroscopy of semiconductor quantum wells
69. 3D coherent spectroscopy of light-harvesting centers
70. 3D coherent frequency domain spectroscopy
71. Two-dimensional spectroscopy of semiconductor quantum dots
72. Optical and electronic properties of quantum dots
73. 2D coherent spectroscopy of GaAs quantum dots
74. 2D spectroscopy of self-assembled In(Ga)As quantum dots
75. Coherent control of quantum dots
76. Coherent control within an ensemble of quantum dots
77. Coherent control of interactions between individual quantum dots
78. Two-dimensional spectroscopy of colloidal quantum dots
79. Two-dimensional spectroscopy of atomically thin 2D materials
80. Introduction to 2D materials
81. Homogeneous linewidth in 2D materials
82. Valley coherence and coupling in 2D materials
83. Other applications of multi-dimensional coherent spectroscopy in Physics
84. Semiconducting carbon nanotubes
85. Color centers in diamond
86. Perovskite materials
87. New trends in multidimensional coherent spectroscopy
88. Broadening the spectral range: from terahertz to x-rays
89. THz MDCS
90. Improving the spatial resolution
91. Multidimensional spectroscopy with quantum light

 

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